Toad appears in 16 issues in this volume.
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Issue #4
The Brotherhood of Evil Mutants
March 1, 1964
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Issue #5
Trapped: One X-man!
May 1, 1964
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Issue #6
Submariner Joins the Evil Mutants
July 1964
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Issue #7
The Return of the Blob
September 1, 1964
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Issue #11
The Triumph of Magneto!
May 1, 1965
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Issue #18
If Iceman Should Fail!
March 1, 1966
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Issue #43
The Torch Is Passed...!
April 1, 1968
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Issue #44
Red Raven,Red Raven
May 1, 1968
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Issue #45
When Mutants Clash
June 1968
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Issue #59
Do or Die, Baby!
August 1, 1969
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Issue #60
In the Shadow of Sauron
September 1969
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Issue #70
...And None Shall Survive! -- If Iceman Should Fail!
June 1, 1971
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Issue #91
X-Men Vs. The Power Of Magneto
December 1, 1974
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Issue #92
Red Raven Lives Again!
February 1, 1975
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Issue #93
When Mutants Clash!
April 1, 1975
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Issue #138
Elegy
October 1980
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