George Klein appears in 53 issues in this volume.
The Boy Witch Doctor!
Stranded in Evolution Valley! / Jimmy Olsen in Scotland Yard! / Jimmy Olsen, Freak!
The Fantastic Army of General Olsen!
Jimmy Olsen's Wildest Adventure!
June 1, 1962
Superman's Phantom Pal
July 1, 1962
The League of Fantastic Supermen
September 1, 1962
Jimmy Olsen, Hollywood Star! / Jimmy Olsen's Fiery Friends! / Jimmy Olsen's Super-Romance!
The Human Porcupine!
The Cabinet from Krypton
January 1, 1963
The Dummy that Haunted Jimmy Olsen! / Leslie Lowe, Girl Reporter! / Super Lucy Lane!
The Helmet of Hate!
The Dynamic Duo of Kandor!
The Secret of Silver Kryptonite!
July 1, 1963
The Plot Against Olsen! ; Jimmy Olsen Meets Cleopatra!
September 1, 1963
The World Of Doomed Olsens!
October 1, 1963
The Kid with the Golden Touch!
December 1, 1963
The Pranks of Jimmy the Imp!
January 1, 1964
The Mystery of Convict 313! / The Voyage of the Mary Celeste II! / When Supergirl Replaced Jimmy Olsen!
Elastic Lad Jimmy And His Legion Romance!
April 1, 1964
The Colossus of Metropolis!
June 1, 1964
The Revenge of Jimmy Olsen!
July 1, 1964
The Red-Headed Beatle of 1,000 B.C.!
September 1, 1964
The Bizarro Jimmy Olsen! / Jimmy Olsen's Double-Trouble!
The Ransom of Superman! / The Demons from Pandora's Box! / Jimmy's Indian Super-Pal!
Jimmy Olsen's Magic Gloves! / The Wedding of Magi and Sandra! / The Unbeatable Jimmy Olsen
Jimmy Olsen's Captive Double!
March 1, 1965
Jimmy Olsen's Monster Movie!
April 1, 1965
King Olsen's Private Island!
June 1, 1965
The Team of Olsen and Brainiac!
July 1, 1965
The Arena of Doom
September 1, 1965
The Swinging Superman! : See Superman Strut the Krypton Crawl!
October 1, 1965
The Brain-Washing of Big Jimmy! / Mr. Mxyzptlk's Partner in Crime!
The Dragon Delinquent!
March 1, 1966
The Batman-Superman of Earth-X! / Sergeant Olsen... Toughest Man in the Marines!
Insect-Olsen versus the Bug Bandits! / The Kid who replaced Jimmy Olsen!
Jimmy Olsen's Greatest Masquerades and His Pal, Superman!
The Prize Is a Planet! : Look Out World... Here Comes Atlas Olsen!
September 1, 1966
The Fortress Death-Trap! / His Highness, Prince Jimmy Olsen!
The Bride of Jungle Jimmy!
December 1, 1966
The One-Man Legion!
January 1, 1967
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