George Klein appears in 54 issues in this volume.
The Boy Witch Doctor!
Stranded in Evolution Valley! / Jimmy Olsen in Scotland Yard! / Jimmy Olsen, Freak!
The Fantastic Army of General Olsen!
Jimmy Olsen's Wildest Adventure!
June 1, 1962
Superman's Phantom Pal! / Jimmy's Duel with Goliath! / Jimmy's Robot Slave!
The League of Fantastic Supermen / Jimmy Olsen, Editor-In-Chief! / The Tom Thumb Jimmy Olsen!
Jimmy Olsen, Hollywood Star! / Jimmy Olsen's Fiery Friends! / Jimmy Olsen's Super-Romance!
The Human Porcupine!
The Cabinet from Krypton
January 1, 1963
The Dummy that Haunted Jimmy Olsen! / Leslie Lowe, Girl Reporter! / Super Lucy Lane!
The Helmet of Hate!
The Dynamic Duo of Kandor!
The Secret of Silver Kryptonite!
July 1, 1963
The Plot Against Olsen! / Jimmy Olsen Meets Cleopatra! / The Nine Lives of Jimmy Olsen!
The World Of Doomed Olsens!
October 1, 1963
The Kid with the Golden Touch!
December 1, 1963
The Pranks of Jimmy the Imp! / Jimmy Olsen and the Forty Thieves! / Jimmy Olsen's Secret Love!
The Mystery of Convict 313! / The Voyage of the Mary Celeste II! / When Supergirl Replaced Jimmy Olsen!
Elastic Lad Jimmy and His Legion Romance! / The Death March! / The Goose with the Golden Eggs!
The Colossus of Metropolis!
June 1, 1964
The Revenge of Jimmy Olsen!
July 1, 1964
The Red-Headed Beatle of 1,000 B.C.!
September 1, 1964
The Bizarro Jimmy Olsen! / Jimmy Olsen's Double-Trouble!
The Ransom of Superman! / The Demons from Pandora's Box! / Jimmy's Indian Super-Pal!
Jimmy Olsen's Magic Gloves! / The Wedding of Magi and Sandra! / The Unbeatable Jimmy Olsen
Jimmy Olsen's Captive Double!
March 1, 1965
Jimmy Olsen's Monster Movie!
April 1, 1965
Love Me, Love My Beast! / The Adventures of Chameleon-Head Olsen! / King Olsen's Private Island!
Jimmy Olsen, Ape Man / Jimmy's D-Day Adventure! / The Team of Olsen and Brainiac!
The Arena of Doom
September 1, 1965
The Swinging Superman! : See Superman Strut the Krypton Crawl!
October 1, 1965
The Infamous Four! / Olsen's Super-Survival Kit!
The Brain-Washing of Big Jimmy! / Mr. Mxyzptlk's Partner in Crime!
The Dragon Delinquent!
March 1, 1966
The Batman-Superman of Earth-X! / Sergeant Olsen... Toughest Man in the Marines!
Insect-Olsen versus the Bug Bandits! / The Kid who replaced Jimmy Olsen!
Jimmy Olsen's Greatest Masquerades and His Pal, Superman!
The Prize Is a Planet! : Look Out World... Here Comes Atlas Olsen!
September 1, 1966
The Fortress Death-Trap! / His Highness, Prince Jimmy Olsen!
The Bride of Jungle Jimmy!
December 1, 1966
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