Metropolis appears in 113 issues in this volume.
Jimmy Olsen's Secret Power
The Son of Jimmy Olsen!
October 1, 1961
The Boy Witch Doctor!
Stranded in Evolution Valley! / Jimmy Olsen in Scotland Yard! / Jimmy Olsen, Freak!
The Fantastic Army of General Olsen!
Superman's Phantom Pal
July 1, 1962
Jimmy Olsen, Hollywood Star! / Jimmy Olsen's Fiery Friends! / Jimmy Olsen's Super-Romance!
The Human Porcupine!
The Cabinet from Krypton
January 1, 1963
The Dummy that Haunted Jimmy Olsen! / Leslie Lowe, Girl Reporter! / Super Lucy Lane!
The Helmet of Hate!
The Secret of Silver Kryptonite!
July 1, 1963
The World Of Doomed Olsens!
October 1, 1963
The Kid with the Golden Touch!
December 1, 1963
The Pranks of Jimmy the Imp!
January 1, 1964
The Mystery of Convict 313! / The Voyage of the Mary Celeste II! / When Supergirl Replaced Jimmy Olsen!
Elastic Lad Jimmy And His Legion Romance!
April 1, 1964
The Colossus of Metropolis!
June 1, 1964
The Red-Headed Beatle of 1,000 B.C.!
September 1, 1964
The Bizarro Jimmy Olsen! / Jimmy Olsen's Double-Trouble!
The Ransom of Superman! / The Demons from Pandora's Box! / Jimmy's Indian Super-Pal!
Jimmy Olsen's Magic Gloves! / The Wedding of Magi and Sandra! / The Unbeatable Jimmy Olsen
Jimmy Olsen's Captive Double!
March 1, 1965
King Olsen's Private Island!
June 1, 1965
The Arena of Doom
September 1, 1965
The Swinging Superman! : See Superman Strut the Krypton Crawl!
October 1, 1965
The Brain-Washing of Big Jimmy! / Mr. Mxyzptlk's Partner in Crime!
The Batman-Superman of Earth-X! / Sergeant Olsen... Toughest Man in the Marines!
Insect-Olsen versus the Bug Bandits! / The Kid who replaced Jimmy Olsen!
The Fortress Death-Trap! / His Highness, Prince Jimmy Olsen!
The Bride of Jungle Jimmy!
December 1, 1966
Superman's Greatest Double-Cross! / Jimmy Olsen - - Campus Hero!
The Murder of Clark Kent!
July 1, 1967
The World of 1,000 Olsens!
The Lone Wolf Legionnaire Reporter! / Superman's Unluckiest Day!
The Rise and Fall of Superman! / The Captive of the Spidermen!
The Midas of Metropolis! / Jimmy Olsen, the Boy Swordsman!
Luthor's Pal, Jimmy Olsen! / The Human Octopus!
The Murderous Magnaman! / Jimmy the Red, Thor's Best Pal!
Survival of the Fittest! / The Kid who unmasked Superman!
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