I think catwoman would work because opposites attract. That's why the Batman/Catwoman thing has always worked it's grounded in reality. Batman at the end of TDK was on the run and this would lead him into a relationship with her. She is a criminal but has a good heart at the core.
This brings me back to one of my favorite storylines...Hush. I believe Nolan could us Hush like he did Ra's in the Batman Begins...with a twist and a big reveal. The more Nolan plays with Batman's head the better the movie and I don't feel Talia or Riddler would bring the same shock value or twists that Joker or Ra's did.
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