Here's my list:
Thanos = Mark Rolston [Aliens & The Departed]
Mistress Death = Jennifer Connelly
Silver Surfer = Doug Jones [Why mess with a good thing?]
Drax the Destroyer = Vinnie Jones [X3 : Juggernaut]
Nebula = Sharon Stone
The Champion = Paul Wight [WWE's The Big Show]
The Runner = Ashton Kutcher
The Gardener = Sir Ian McKellan
The Gamesmaster = Sir Anthony Hopkins
The In-Betweener = David Hasselhoff
The Collector = Donald Sutherland
Mephisto = Adrien Brody [The Jacket, King Kong]
Pip the Troll = Danny DeVito
Gamora = Jennifer Garner
Adam Warlock = James Marsters [Spike from Buffy]
Dr Strange = Pierce Brosnan
Wong = Jackie Chan? LOL
Rintrah[CGI?]
Mentor = Terance Stamp [Gen Zod from Superman II]
Eros = Brad Pitt
Firelord[CGI?] Voiced by Keith David (Goliath from Gargoyles & HBO's Spawn)
Dr Doom = Michael York
She-Hulk = Lucy Lawless
WonderMan = Ben Affleck
Scarlet Witch = Famke Jennsen
Iron Man = Timothy Dalton
Hulk = Eric Bana [Again, why mess with CGI beauty?]
Thor = Vladimir Kulich [13th Warrior Leader Buliwyf]
Spider-Man = Toby Maquire [Of course.]
Captain America = Matt Salinger [One more try, but w/ a big budget]
Cloak = Michael Clarke Duncan
Sersi = Katie Holmes [Small part and she needs the work]
Black Knight = Sean Bean [LOTR's Boromir]
Wolverine = Hugh Jackman [Yeah, baby! SNIKT!]
Cyclops = Matt Damon [James Marsden SUCKS! as Cyclops]
Namor = The Rock
Nova = Brendan Frazer [The Mummy]
Quasar = Seth Green
Kree Commander = Dolph Lundgren
Skrull Commander = Eric Roberts
Odin = Brian Blessed [Prince Voltan [Hawkmen] from Flash Gordon 1980]
Terraxia = Shae Marks [Playmate March 1992]
Eternity [CGI?] Voiced by Viggo Mortensen [LOTR's Aragorn]
Living Tribunal [CGI?] Voiced by Kevin Conroy (Animated Batman) but tri-voiced like the Transformers
Galactus = Orson Wells (Hey, if they can get Brando from the grave why not Wells?)
Uatu the Watcher = Ben Kingsley
Mistress Love = Jessica Simpson
Sire Hate = Chyna [Formerly WWE]
Chaos & Order [CGI?]Voiced by Kevin Michael Richardson [both]
Celestials [CGI?]
Epoch [CGI?] Voiced by John Rys-Davies [LOTR's Gimli/Treebeard]
Kronos
Teasers:
Magus [Warlock] = James Marsters [Spike from Buffy]
Goddess [Warlock] = Elizabeth Shue
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