Dr. Wily. Despite always being the bad guy in any Mega Man game, he always somehow convinces the world that he's changed his evil ways before being revealed as the villain at the end. :P
Even though he's a comic book villain primarily, originally, and first and foremost. :P
Best video game villains for me would have to be Ganondorf, the Covenant from HALO, Ridley, all the gym leaders from the old pokemon games (rock gym leader as the first gym leader in a game where you get an electric pokemon first? Lolhax)
A neat alternate videogame villain (i.e. character who wasn't a villain, but would make an amazing villain), is Auron from FF10. He'd be like Wesker, only for FF10; calm, cool, badass, treacherous, uber powerful, makes people cower in fear on-demand, sleek hair...
EDIT: Turns out I already posted in this thread. Derp. I agree with my original post in here mostly, Ganondorf and Ridley are still some of my favorites, but Lavos is also one of my favorites. The Covenant don't really count I guess, they're an organization, and become allies later on, so they're kind of in the air.
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