Lex Luthor would be awesome. Perhaps it can show his life's difficulties and his hard work to success that would ultimately cause his hate towards Superman and "aliens" and his belief that only man can succeed and can't depend on an alien like Supes.
Black Adam would be awesome as well, showing his beginnings in the past after getting the powers of the gods for the first time; his downfall from Adam the "Great" to "Black Adam"; the cause of his disappearance for years and years; his rule over Kahndaq with his iron fist; his love for Iris leading him to become allies with the Justice League as an anti-hero-kinda; and, eventually in/slightly before the last act, Iris's death causing him to turn evil again.
Any supervillain team up in Marvel/DC such as Sinister Six, Injustice League, Legion of Doom, or Suicide Squad, etc.
Dr. Doom is pretty much undeniable; that movie would be awesome.
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