Artie Simek appears in 55 issues in this volume.
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Issue #2
The Evil Menace of Electro!
June 1, 1964
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Issue #3
The Owl, Ominous Overlord of Crime!
August 1, 1964
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Issue #7
In Mortal Combat With... The Sub-Mariner!
April 1965
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Issue #10
While the City Sleeps!
October 1, 1965
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Issue #14
If this Be Justice...!
March 1, 1966
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Issue #15
And Men Shall Call Him...Ox!
April 1, 1966
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Issue #16
Enter... Spider-Man!
May 1, 1966
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Issue #21
The Trap is Sprung
October 1, 1966
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Issue #22
The Tri-Man Lives!
November 1, 1966
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Issue #23
DD Goes Wild!
December 1, 1966
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Issue #24
The Mystery of the Midnight Stalker!
January 1, 1967
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Issue #25
Enter: The Leap Frog!
February 1, 1967
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Issue #26
Stilt-Man Strikes Again
March 1, 1967
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Issue #27
Mike Murdock Must Die!
April 1, 1967
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Issue #30
If There Should Be A Thunder God!
July 1, 1967
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Issue #31
Blind Man's Bluff!
August 1, 1967
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Issue #33
Behold... The Beetle!
October 1, 1967
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Issue #34
To Squash A Beetle!
November 1, 1967
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Issue #35
Daredevil Dies First!
December 1, 1967
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Issue #36
The Name of the Game is Mayhem!
January 1968
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Issue #37
Don't Look Now, But It's... Dr. Doom!
February 1, 1968
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Issue #39
The Exterminator And The Super-Powered Unholy Three
April 1, 1968
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Issue #43
In Combat With Captain America!
August 1, 1968
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Issue #44
I, Murderer!
September 1, 1968
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Issue #45
The Dismal Dregs of Defeat!
October 1, 1968
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Issue #46
The Final Jest
November 1, 1968
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Issue #47
Brother, Take My Hand!
December 1, 1968
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Issue #48
Farewell To Foggy!
January 1, 1969
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Issue #49
Daredevil Drops Out
February 1, 1969
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Issue #51
Run, Murdock, Run!
April 1, 1969
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Issue #53
As It Was In The Beginning...
June 1, 1969
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Issue #56
...And Death Came Riding
September 1969
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Issue #57
In The Midst Of Life...!
October 1, 1969
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Issue #59
The Torpedo Will Get You You If You Don't Watch Out!
December 1, 1969
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Issue #62
Quoth The Nighthawk, 'Nevermore!'
March 1, 1970
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Issue #63
The Girl... Or The Gladiator?
April 1, 1970
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Issue #64
Suddenly... The Stunt-Master!
May 1, 1970
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Issue #65
The Killing Of Brother Brimstone
June 1, 1970
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Issue #66
...And One Cried Murder!
July 1, 1970
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Issue #67
Stilt-Man Stalks The Soundstage
August 1, 1970
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