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Once perhaps the most evil vampire in the world, Angel regained his soul after being cursed by gypsies for killing one of their young women, and set out to redeem himself by helping others.
Born of two vampires, this human teen is truly formidable. The first "dhampir" of the Whedon-verse Connor has been alluded to be some form of savior.
Charles Gunn was a vampire hunter, member of Angel Investigations and, for several months, head of the legal department at Wolfram & Hart Los Angeles branch, until the rebellion of Team Angel. He was temporarily turned into a vampire after the fall of LA.
Fred Burkle was saved from another dimension by Angel Investigations. She joined up and worked with them for years, until her soul was destroyed and her body taken over by the Demon Old One, Illyria.
An infamous vampire, Spike began to help Buffy in her fight once he could no longer bite humans. Later, he fought to get his soul back so that Buffy could love him, and sacrificed himself for her.
Wesley Wyndam-Pryce was a British former Watcher and, later, key member of Angel Investigations. Wesley later becomes a reluctant spiritual employee of Wolfram & Hart. He was killed trying to defeat the evil Cyvus Vail, a powerful demonic warlock.
Gwen is a human with electrical powers.
Former LA police officer pulled into the world of Angel. After leaving the force, she opens an antique store to learn more about mystical things.
At first James was a Potentate, warrior angel of the Powers That Be and an ally of Angel. But then, is revealed that is a demonic higher being decided to conquer the human world after he purchased it from his sister.
Angel's Dragon was freed during the fight after the fall. Angel keeps her name secret for quite a while, before telling it to his son Connor to use as a sign the Dragon should trust him. After hearing her name, Cordelia gives Connor the same allegiance given his father.
Eddie Hope, a devil who seeks revenge after returning from the hell of L.A., after of the events of "After the Fall".
Beta George is a fish with telepathic abilities.
A she-jaguar shapeshifter.
Laura Weathermill was a member of the Watchers' Council and later a member of Angel Investigations.
Lorne is an empath demon from another dimension, a good demon who enjoys music more than mayhem. He has guest-starred in Angel and Angel spinoff comics from time to time.
The champion Pylea, the Groosalugg fell in love with Cordelia Chase, and fought against, and later with, Angel and Angel Investigations for her love.
Nina Ash is a young woman who was attacked by a werewolf. Therefore, she turned into a werewolf and Angel did help her to cope with her situation.
Mr. Polyphemus was a Monasterenser Magnaserm partnered with Angel Investigations member, and ex-Watcher, Laura Kay Weathermill.
Anne Steele (born Joan and formerly known as Sister Sunshine, Chantarelle and Lily Houston) was a social worker and the director of the East Hills Teen Center in Los Angeles.
A Soul Eater raised by James to destroy Angel and Spike.
Rowant Mor is Myr's sister, big bad of IDW's Angel comics.
She was once leader of a clique of girls called "the Cordettes". Then she became a cheerleader, an actress, a conduit to the Powers that Be, part demon, a champion, and finally a Higher Power. Cordelia Chase was the heart (and wit) of Angel Investigations.
Burge is the Lord of Downtown L.A.
Tiny Illyria's friend.
Bro'os is the Lord of Santa Monica.
Winifred "Fred" Burkle is a Texan who moved to LA to study physics. After being abducted from LA to the dimension of Pylea and returned, she joined Angel Investigations, becoming well known for her compassion, intellect and innocence, something that she did exploit thoroughly.
Kr'ph is the Lord of Westwood
Drusilla was the love of Spike the vampire for several hundred years, and was also Spike's sire. She was tormented emotionally and psychologically before dying, eventually to become an insane vampire who had visions of the future.
Maria Harley, a.k.a. Spider, a demon and ally of Spike and Angel Investigations.
Holland Manners was a high-ranking lawyer and executive at Wolfram & Hart, one of the top servants of the Senior Partners.
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